The SNES could put out some great sound. I loved the music in Gradius III. Seems it was much easier to get decent voice from it vs. the Genesis. On, the downside, I found a lot of stuff was kinda muffled, though.
The high point of Genesis audio (for me) was the Thunderforce series. They could pound out some rock'n tunes from that thing!
My personal preference would be Genesis audio with better voice sampling.
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